Mechanistic insights into dual active sites in Au@W<sub>18</sub>O<sub>49</sub> electrocatalysts for the hydrogen evolution reaction

Yu, Yaqin; Zhou, Zhen; Song, Xiaoping; Song, Xiaowei; Zhang, Zhengdong; Jing, Chuanyong

doi:10.1039/d2qi00993e

Cited by 3 publications

(1 citation statement)

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“…Heretofore, adsorption, ion exchange, biological method, advanced oxidation processes (AOPs) have been employed as instrumentalities for UDMH polluted wastewater purification. Nevertheless, the practical application of above methods were hindered by their inherent demerits [3,[6][7][8][9].…”

Section: Introductionmentioning

confidence: 99%

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Zhou¹,

Zheng²,

Li³

et al. 2023

Pol. J. Environ. Stud.

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Releasing unsymmetrical dimethyl hydrazine (UDMH) in ambient medium is an escalating environment crisis that catches aggrandizing public concerns. Herein, a non-thermal plasma activating persulfate maneuver was introduced and its application mechanism in UDMH degradation was explored.Oxidizing kinetic experiments show that 93.8% UDMH were eliminated along with 12.5 kV, pH = 8, 50 mM NaCl, Na 2 S 2 O 8 /UDMH (mol/mol) = 2, and 140 mL/min. The Visual MINTEQ simulated species distribution of UDMH well predicted the oxidation behaviors of UDMH in the variation of pH. Radical scavenging test integrated with UV-vis spectroscopy were introduced to identify the predominating reactive oxygen species during UDMH decomposition. The •OH and •SO 4 played a synergistic role in the UDMH oxidization. Overall, this study may shed new lights on the degradation of UDMH industry wastewater using hybrid technique.

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Section: Introductionmentioning

confidence: 99%

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Zhou¹,

Zheng²,

Li³

et al. 2023

Pol. J. Environ. Stud.

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show abstract

Comparative study on the effects of {2 0 1} TiO2 and {2 0 1}TiO2−ZrO2 on arsenite photocatalysis

Zhou¹,

Fang³

et al. 2023

Inorganic Chemistry Communications

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Self-supported Ni-NiWO4@NC heterojunction as high-efficient electrocatalyst for overall water splitting

Kong,

Fang,

Wang

et al. 2024

Journal of Alloys and Compounds

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Mechanistic insights into dual active sites in Au@W₁₈O₄₉ electrocatalysts for the hydrogen evolution reaction

Abstract: Electrocatalytic hydrogen evolution reaction (HER) for water splitting is promising to replace fossil fuels. The high-efficient electrocatalyst with multiple functional sites is indispensable but challenging. Herein, urchin-like Au@W18O49 electrocatalyst with...

Cited by 3 publications

References 38 publications

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Comparative study on the effects of {2 0 1} TiO2 and {2 0 1}TiO2−ZrO2 on arsenite photocatalysis

Self-supported Ni-NiWO4@NC heterojunction as high-efficient electrocatalyst for overall water splitting

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Mechanistic insights into dual active sites in Au@W18O49 electrocatalysts for the hydrogen evolution reaction

Abstract: Electrocatalytic hydrogen evolution reaction (HER) for water splitting is promising to replace fossil fuels. The high-efficient electrocatalyst with multiple functional sites is indispensable but challenging. Herein, urchin-like Au@W18O49 electrocatalyst with...

Cited by 3 publications

References 38 publications

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Activated Persulfate by Dielectric Barrier Discharge Plasma for the Degradation of Unsymmetrical Dimethyl Hydrazine as Wastewater Pollutants

Comparative study on the effects of {2 0 1} TiO2 and {2 0 1}TiO2−ZrO2 on arsenite photocatalysis

Self-supported Ni-NiWO4@NC heterojunction as high-efficient electrocatalyst for overall water splitting

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Mechanistic insights into dual active sites in Au@W₁₈O₄₉ electrocatalysts for the hydrogen evolution reaction