[1] Aircraft measurements of cloud condensation nuclei (CCN) and microphysics of clouds at various altitudes were conducted over India during CAIPEEX (Cloud Aerosol Interaction and Precipitation Enhancement Experiment) phase I and II in 2009 and 2010 respectively. As expected, greater CCN concentrations gave rise to clouds with smaller drops with greater number concentrations (N c ). The cloud drop effective radius (r e ) increased with distance above cloud base (D). Warm rain became detectable, i.e., rain water content >0.01 g/Kg, at the tops of growing convective clouds when r e exceeded 12 mm. The r e is determined by the number of activated CCN, N ad , and D. The N ad can be approximated by the maximum measured values of N c . Higher N c resulted in greater D for reaching the r e threshold for onset of warm rain, r e *, denoted as D*. In extreme cases of highly polluted and moist air that formed the monsoon clouds over the Indo-Gangetic plains, D* exceeded 6 km, well above the 0 C isotherm level. The precipitation particles were initiated there as supercooled raindrops at a temperature of À8 C. Giant CCN reduced r e * and D*, by initiating raindrops closer to cloud base. This effect was found mainly in dusty air masses over the Arabian Sea. Besides, the aerosol effect on D*, D* was found to decrease with increase in cloud water path.