We account for dynamical spin effects in the holographic light-front wavefunction of the pion in order to predict the mean charge radius, r 2 π , the decay constant, f π , the spacelike electromagnetic form factor, F π (Q 2 ), the twist-2 pion Distribution Amplitude and the photon-to-pion transition form factor F γπ (Q 2 ). Using a universal fundamental AdS/QCD scale, κ = 523 MeV, and a constituent quark mass of 330 MeV, we find a remarkable improvement in describing all observables.