Metallic Cu-incorporated NiFe layered double hydroxide nanosheets enabling energy-saving hydrogen generation from chlorine-free seawater electrolysis coupled with sulfion upcycling

Jiang, Jing; Tian, Yao; Zhang, Jiayi; Zhang, Chenghui; Ai, Lunhong

doi:10.1016/j.fuel.2024.131506

Fuel

2024

DOI: 10.1016/j.fuel.2024.131506

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Metallic Cu-incorporated NiFe layered double hydroxide nanosheets enabling energy-saving hydrogen generation from chlorine-free seawater electrolysis coupled with sulfion upcycling

Jing Jiang,

Yao Tian,

Jiayi Zhang

et al.

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Cited by 6 publications

References 62 publications

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Partially Amorphous Ru‐Doped CoSe Nanoparticles with Optimized Intermediates Adsorption for Highly Efficient Sulfur Oxidation Reaction

Liu,

Wang,

Wan

et al. 2024

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The application of thermodynamically more favorable sulfur oxidation reaction (SOR) to replace oxygen evolution reaction (OER) in electrocatalytic water electrolysis is an appealing strategy to achieve low‐energy hydrogen production while removing toxic sulfur ions from wastewater. However, the study of SOR catalysts with both activity and stability still faces great challenges. Herein, this study prepares partially amorphous Ru‐doped CoSe (pa‐Ru‐CoSe) nanoparticles for SOR. The doping of Ru keeps Co in an electron‐deficient state, which enhances the adsorption of SOR intermediates and improves the catalytic activity. Meanwhile, the partially amorphous selenide possesses great corrosion resistance to sulfur species, thus ensuring stability in long‐term SOR. In addition, the pa‐Ru‐CoSe requires only 0.566 V to reach a current density of 100 mA cm−2 in the SOR‐HER coupled system and remains stable for 200 h. This work provides a promising partially amorphous strategy for SOR catalysts with both catalytic activity and long‐term stability, enabling hydrogen production with low energy consumption and simultaneous sulfur production.

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Partially Amorphous Ru‐Doped CoSe Nanoparticles with Optimized Intermediates Adsorption for Highly Efficient Sulfur Oxidation Reaction

Liu,

Wang,

Wan

et al. 2024

Small

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CoNiOOH nanosheets array enables highly effective value-added chemicals production via nitrite and sulfide electrolysis

Yang,

Wei,

Zeng

et al. 2024

Chemical Engineering Journal

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Energy-saving hydrogen production from sulfion oxidation-hybrid seawater splitting enabled by superwettable corrosion-resistant NiFe layered double hydroxide/FeNi2S4 heterostructured nanoarrays

Ai,

Tian,

Xiao

et al. 2024

Journal of Colloid and Interface Science

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Metallic Cu-incorporated NiFe layered double hydroxide nanosheets enabling energy-saving hydrogen generation from chlorine-free seawater electrolysis coupled with sulfion upcycling

Cited by 6 publications

References 62 publications

Partially Amorphous Ru‐Doped CoSe Nanoparticles with Optimized Intermediates Adsorption for Highly Efficient Sulfur Oxidation Reaction

Partially Amorphous Ru‐Doped CoSe Nanoparticles with Optimized Intermediates Adsorption for Highly Efficient Sulfur Oxidation Reaction

CoNiOOH nanosheets array enables highly effective value-added chemicals production via nitrite and sulfide electrolysis

Energy-saving hydrogen production from sulfion oxidation-hybrid seawater splitting enabled by superwettable corrosion-resistant NiFe layered double hydroxide/FeNi2S4 heterostructured nanoarrays

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