2024
DOI: 10.1002/ange.202405252
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Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling

Jiayou Feng,
Jindi Duan,
Chin‐Te Hung
et al.

Abstract: Catalytic upcycling of polyolefins into high‐value chemicals represents the direction in end‐of‐life plastics valorization, but poses great challenges. Here, we report the synthesis of a tandem porous catalyst via a micelle cascade assembly strategy for selectively catalytic cracking of polyethylene into olefins at a low temperature. A hierarchically porous silica layer from mesopore to macropore is constructed on the surface of microporous ZSM‐5 nanosheets through cascade assembly of dynamic micelles. The out… Show more

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