2017
DOI: 10.1002/2016gl072486
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Microscale characteristics of homogeneous freezing events in cirrus clouds

Abstract: We investigate homogeneous freezing of aqueous aerosol particles, a fundamental ice formation process in cirrus clouds. We estimate freezing time scales and vertical extensions of freezing layers, demonstrating that such freezing events are highly transient and localized. While time scales decrease with increasing vertical velocity driving ice nucleation, layer depths are weak functions of the vertical velocity. Our results are used to discuss possible effects of turbulent diffusion and entrainment‐mixing on h… Show more

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Cited by 12 publications
(16 citation statements)
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“…The simulations capture the dependence of nucleated ICNC on the homogeneous freezing temperature, T ⋆ , which is, however, very weak. We note that across all the cases discussed here, T * ≈218 K with very little scatter (±0.25 K), corresponding to a narrow range of ice saturation ratios, S ⋆ ≈1.5 ± 0.02, characteristic for homogeneous freezing events (Kärcher & Jensen, ). Examining the full upper tropospheric temperature range would reveal significant variations of T ⋆ and nucleated ICNC.…”
Section: Stochastic Simulationsmentioning
confidence: 75%
“…The simulations capture the dependence of nucleated ICNC on the homogeneous freezing temperature, T ⋆ , which is, however, very weak. We note that across all the cases discussed here, T * ≈218 K with very little scatter (±0.25 K), corresponding to a narrow range of ice saturation ratios, S ⋆ ≈1.5 ± 0.02, characteristic for homogeneous freezing events (Kärcher & Jensen, ). Examining the full upper tropospheric temperature range would reveal significant variations of T ⋆ and nucleated ICNC.…”
Section: Stochastic Simulationsmentioning
confidence: 75%
“…They interpreted these changes as being an effect of more frequent heterogeneous freezing on aviation exhaust particles. It has long been known that aircraft-emitted particles may act as efficient ice nuclei, leading to heterogeneous nucleation in regions with a favorable atmospheric state (including temperature and humidity) (e.g., Schumann, 1996;Jensen and Toon, 1997;Kärcher, 2007). Furthermore, aviation-induced aerosols and contrails can alter the properties of cirrus clouds (e.g., Tesche et al, 2016;Kärcher, 2017;Urbanek et al, 2018).…”
mentioning
confidence: 99%
“…As illustrated in Figure , we make the assumption that the presence of cloud ice constrains q v locally to ice saturation, that is, q v ≃ q s . This does not hold during short‐term ice formation events (Kärcher & Jensen, ). For the purpose of this study, we identify the vapor PDF with a delta distribution: PDFfalse(qvfalse)=δfalse(qvqsfalse(Tfalse)false)0.3em. …”
Section: Resultsmentioning
confidence: 97%
“…As illustrated in Figure 1, we make the assumption that the presence of cloud ice constrains q v locally to ice saturation, that is, q v ≃ q s . This does not hold during short-term ice formation events (Kärcher & Jensen, 2017).…”
Section: Total Water Statisticsmentioning
confidence: 99%