In this paper, the effect of ceramic particles (Zirconium, Boron Carbide and Graphene) on the ballistic resistance of Friction Stir Processed (FSPed) thick AA6061 targets had been explored. The Base Metal AA6061 plates of 25 mm thickness were FSPed by reinforcing Zirconium (Zr), Boron Carbide (B4C) and Graphene (G), thus producing FSPed-Zr, FSPed-B4C and FSPed-G surface composite targets. Microhardness test was carried out and the hardness of FSPed-Zr, FSPed-B4C and FSPed-G were found to be 96, 106 and 122 HV respectively. High velocity ballistic experiments were conducted on all the targets against Ø7.62x51 mm Armour Piercing Projectile at an initial velocity of 680 ± 10 m/s. AA6063 backing plates were used to identify the ballistic resistance of the FSPed targets by Depth of Penetration (DOP) method. Consequently, higher microhardness along with frictional characteristics had increased the ballistic resistance of FSPed-G targets by 70.8%. Further, by analyzing the penetration channel, it was noticed that in FSPed-G target, the jacket detachment occurred in the entry region predominantly where the microhardness was the highest compared to other two regions. This phenomenon occurred just after the entry region for FSPed-B4C target and in middle region for FSPed-Zr target. Scanning Electron Microscopy (SEM) images inferred that, FSPed targets have absorbed maximum projectile’s kinetic energy at the entry region itself, resulting in formation of cracks. As a result, middle and exit region experienced less impact. Post ballistic microhardness test showed enhanced microhardness in the entry region of FSPed-G target due to severe work hardening. Hence the ceramic particles deposited by FSP have reduced the kinetic energy of the projectile with FSPed-G target resulting in maximum ballistic resistance.