“…Significantly, the as-assembled Ni-Fe device in the present work shows the highest energy density of 235.2 W h kg À1 (19.6 W h cm À3 ) at a power density of 540.7 W kg À1 (45 W cm À3 ) and still retains a high power density of 5.4 kW kg À1 (450 W cm À3 ) at an ultrahigh energy density of 82 W h kg À1 (6.8 W h cm À3 ). The values are comparative to those of the previously reported aqueous energy storage devices, 55,56 such as GF/CNTs/Ni(OH) 2 //GF/ CNTs/-Fe 2 O 3 , 57 p-MG//p-FG, 58 NiCo 2 O 4 /NiO//Fe 2 O 3 , 59 NiNTAS@ Fe 2 O 3 //NiNTAS@MnO 2 , 60 MoO 3 @CNT//MnO 2 @CNT, 61 Ni 0.1 Co 0.9 -Se 2 @NF//rGO@NF 62 and are even comparable to some of the aqueous Ni-Fe batteries (see Table S2, ESI †), such as Ni(OH) 2 MSs@NF//Fe 2 O 3 @GH battery (203 W h kg À1 at 0.798 kW kg À1 ), 47 NiO@C//Fe@C (138 W h kg À1 at 0.61 kW kg À1 ), 63 Ni-Co DH/OG// Fe 3 O 4 /FeOOH/OG (161.3 W h kg À1 at 5.7 kW kg À1 ), 64 and Ni@CMFs//Fe@CMFs (116 W h kg À1 at 5.76 kW kg À1 ). 65 The device also shows a good cycling stability of 81.2% (Fig.…”