Accurate estimation of mineral composition is essential for refined reservoir characterization, thermal conductivity and mechanical determinations of sedimentary rocks, but is extremely challenging in shale units due to the mineralogical complexity, low porosity and ultra‐low permeability. Direct mineral measurements derived from laboratory X‐ray diffraction (XRD) analysis on core samples and borehole geochemical logging tool (GLT), and conventional geophysical logs from vertical wells penetrating sediments are widely available in some basins, which enables detailed mineralogical characterization of a well. A hybrid machine learning (ML) architecture that improves model training and validation by combining convolutional neural network (CNN) with XGBoost allows accurate description of the mineralogical compositions across a basin. We applied this ML approach to predict the mineral compositions using conventional well logs from the Horn River Basin, northeast British Columbia, Canada, where extensive drilling for shale‐gas and conventional hydrocarbon resources, complemented by high temperature geothermal energy potential is ideal for case testing. The predicted mineral compositions from the ML approach are consistent with the mineralogical readings from the GLT and are confirmed by the XRD mineral measurements. This allows basin‐wide mineral compositions mapping that reveals spatial trends of major mineral compositions and their relationship with the previously recognized geomechanical and geological features, which have important implications for thermal conductivity modeling, reservoir evaluation and extensive geological studies.