Mise en evidence d'un isotope leger de rubidium

Chaminade, R.; Cros, M.; Gratot, I.; Pape, M. Le

doi:10.1016/0029-5582(57)90075-5

Cited by 14 publications

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“…A large number of energy sum relations, which fit very accurately, indicate that most of these y-rays, including all those of high intensity, are emitted by the same nuclide. There is no reason to doubt that this activity is due to 79 Rb, to which nuclide it is normally ascribed [1,2], although our half-life value is rather longer than the recent one of 20.9 + 0.8 minutes, reported by CHACKETT et al The 6 minutes activity must be due to a nuclide of mass less than 79. In irradiations with 3 He ions of 36 MeV its y-ray spectrum is barely observed, but at 40 MeV it is quite evident, even though still very Table 2 weak.…”

contrasting

confidence: 51%

The Decay of Rubidium-78 and Rubidium-79

Toeset¹,

Jb²

1968

Radiochimica Acta

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Irradiation of bromine with. 3 He ions in the 36 to 72 MeV range has produced a rubidium fraction which, apart from the well known activities of 82m Rb, 81 Rb and 81m Rb, shows activities with half lives of 24 + 2 minutes and 6 + 1 minutes. The former period represents 79 Rb, whereas the 6-minutes period is ascribed to 78 Rb. Quantities of 20 mg ammoniumbromide (p. a. Union Chimique Beige, S. A.) were packed in 0.01 mm gold foil and irradiated for 1 minute with 3 He ions in the synchrocyclotron of this institute. After activation the material was dissolved in water. Both Rbl and Na 2 S0 3 were added, followed by HC10 4 . The RbC10 4 formed was collected by filtration. Counting was started approximately 5 minutes after the irradiation. It was performed with a 20 cm 3 -Ge(Li)detector (Nuclear Diodes) coupled to a Tennelec TC-130 ΓΕΤ charge amplifier, a Tennelec TC-200 linear amplifier and either a Laben-4096 channel analyzer or a PDP-8 (DEC) programmed to act as a multichannel analyzer with a Nuclear Data 4096 ADC. Energy and intensity calibrations of the detector were performed with a set of standard IAEA gammasources. A 2.0 cm perspex absorber or a 1.2 cm lead absorber covered with cadmium and copper were used.The y-rays of the 24 minutes activity are shown in Table 1. This activity was produced in good strength in the whole energy range used for the 3 He ions, i. e. from 36 to 72 MeV. A large number of energy sum relations, which fit very accurately, indicate that most of these y-rays, including all those of high intensity, are emitted by the same nuclide. There is no reason to doubt that this activity is due to 79 Rb, to which nuclide it is normally ascribed [1, 2], although our half-life value is rather longer than the recent one of 20.9 + 0.8 minutes, reported by CHACKETT et al. [2], Our y-ray of 129.7 keV represents the decay of the 55 seconds isomer of 79 Kr, for which CBEUTZ et al. have reported an energy of 127 keV [3]. The 150 keV y-ray, reported by CHAMINADE et al. [1] as a complex radiation, turns out to consist of lines at 143.5 keV and 146.5 keV with a possible contribution due to 154.8 keV. In this connection it should be mentioned that BLECK et al. have observed a delayed y-ray of 148 keV [4], Our measurements do not, on the other hand, give any indication of a 0.46 MeV level, which was reported in ref. [5].Our results are insufficient for the construction of a complete and reliable decay scheme, but there can be hardly any doubt concerning the existence of the levels in 79 Kr at 146.5 keV, 182.8 keV, 290.4 keV, 533.0 keV, 688.2 keV and 752.1 keV, apart from the metastable state at 129.7 keV. Table 1. Energies, measured half-lives and relative intensities of γ-rays observed in the decay of 24 min ™Rb y-ray intensity Energy T 1/2 (normalized to 100 (keV) (min) for 129 keV) 129.7 ± 0.3 25 + 2 100 143.5 ± 0.5 24 + 1 100 ± 10 146.5 ± 0.5 24 + 1 105 + 10 154.8 ± 0.3 24 ± 2 50 + 7 160.7 + 0.2 24 + 2 60 ± 8 182.8 + 0.2 23 + 2 185 + 15 219.0 + 0.5 22 + 2 12 ± 3 350.2 + 0.5 23 ± 1 80 ± 7 383.5 + 0.5 22 ± ...

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