“…Among them, some Tb-Al binary alloys have been particularly studied by neutron scattering techniques [4,5,6]. From those studies, it was concluded that TbAl 2 shows ferromagnetism at T C = 105 K [4], TbAl is a non-collinear antiferromagnet with T N = 72 K [5], whilst Tb 3 Al 2 is a ferromagnet with T C = 190 K [6]. On the other hand, studies of magnetic properties of other members of the Tb-Al series indicated an antiferromagnetic behaviour at T N = 21 K and 52 K for TbAl 3 and Tb 2 Al, respectively [1,7,8].…”