2022
DOI: 10.5802/crchim.134
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n-selective Tsuji–Trost allylation promoted by a recyclable TSIL-palladium complex

Abstract: The Tsuji-Trost reaction of allylic acetates with nucleophiles is optimized using a taskspecific ionic liquid (TSIL)-palladium complex in a very efficient manner. Several nucleophiles and allylic systems are studied obtaining very high yields of the corresponding products with total nselectivity. The reaction is surveyed employing inexpensive allylic alcohols and 3-acyloxindole derivatives affording the expected allylated molecules after a deacylative process. The robustness of the catalytic system is assessed… Show more

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