Nanoporous anodic aluminum oxide (AAO) is needed for a variety of purposes due to its unique properties, including high hardness, thermal stability, large surface area, and light weight. Nevertheless, the use of AAO in different applications is limited because of its brittleness. A new design of an electrochemical reactor with a vibrating element for AAO nanoporous membranes fabrication is proposed. The vibrating element in the form of a piezoceramic ring was installed inside the developed reactor, which allows to create a high-frequency excitation. Furthermore, mixing and vibration simulations in the novel reactor were carried out using ANSYS 17 and COMSOL Multiphysics 5.4 software, respectively. By theoretical calculations, the possibility to excite the vibrations of five resonant modes at different frequencies in the AAO membrane was shown. The theoretical results were experimentally confirmed. Five vibration modes at close to the theoretical frequencies were obtained in the novel reactor. Moreover, nanoporous AAO membranes were synthesized. The novel aluminum anodization technology results in AAO membranes with 82.6 ± 10 nm pore diameters and 43% porosity at 3.1 kHz frequency excitation and AAO membranes with 86.1 ± 10 nm pore diameters and 46% porosity at 4.1 kHz frequency excitation. Furthermore, the chemical composition of the membrane remained unchanged, and the hardness decreased. Nanoporous AAO has become less brittle but hard enough to be used for template synthesis.