“…(1) observed at higher capillary numbers (Ca ∼ 10 −5 − 10 −4 ), where the condition Ca 1/3 ≪ 1 still holds 13,17,25,26 , remain unexplained. To go beyond the assumption of rigid interfaces, several models have been proposed to account for the elastic and/or viscous behavior of the liquid/air interfaces for both LLD [27][28][29][30] and Frankel 5,31,32 configurations. Because the mechanical response of the interfaces is dictated by the interfacial dynamics of surfactants, most of the models make the assumption of water-insoluble surfactants, for which the complex adsorption-desorption dynamics can be disregarded.…”