Adjusting mechanical behavior and controlling deformation parameters are significant tasks in designing shape memory components. In this paper, an analytical model describes the deformation behavior of NiTi/NiTiCu bi-layer composites under tensile loading. Different deformation stages are considered based on single mechanical behavior at each stage. Closed-form equations are derived for stress-strain variations of bi-layer composites under uniaxial loading-unloading. Bi-layer composites made via the diffusion bonding method from single layers of NiTi alloy with a composition of Ti-50.7 at.% Ni, as an austenitic layer, and Ti-45 at% Ni-5 at% Cu, as a martensitic layer, are produced by the vacuum arc remelting technique. The tensile behavior of single-and bi-layers is investigated by using loadingunloading experiments to find the nominal stress-strain curves. Numerical simulations are also done by employing Lagoudas constitutive model to simulate stress-strain diagrams. The solutions of the analytical method presented are validated by using the numerical simulations as well as the experimental results. With regard to the results obtained from the analytical modeling, the numerical simulations, and the experiments, it is evident that the bi-layer composites with different thickness ratios provide adjustable mechanical behavior that can be considered in different application designs, for example, actuators equipped with shape memory components.