The ability of in-flight icing numerical codes to account for the effects of Supercooled Large Droplets (SLD), which are droplets ranging from 50-1000 µm, is still somewhat limited. Solvers that simulate SLD in in-flight icing treat an ensemble of droplets adopting a macroscopic approach, making use of some heuristic correlations based on experiments or extrapolating SLD behavior from smaller non-SLD droplets. Alternatively, taking a microscopic approach and accurately simulating the physics of individual droplets can lead to higher fidelity models when replacing empirical data. Therefore, developing models of a single SLD droplet impingement and solidification can provide a framework that expands the capabilities of current macroscopic solvers to handle water-ice fluid-structure interactions (FSI) and solidification.This presents challenges such as the evolution of the water-ice interface and the jump in fluid/solid properties due to phase change. This thesis proposes a level set method (LSM) to capture the movement of the interface, and the extended finite element method (XFEM) to sharply account for the discontinuities in the material properties without the need for body-conforming meshes.