2012
DOI: 10.1063/1.3673560
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Modulation of surface plasmon wave by photo-induced refractive index changes of CdSe quantum dots

Abstract: We demonstrate an all-optical modulation of surface plasmon resonance by photo-irradiation induced dielectric constant change of CdSe quantum dots on the gold surface. The dipole-dipole interaction between the surface plasmon and the photo-induced excitons in the dots gives rise to a shift in the surface plasmon resonance peak. This shift is found to sensitively reflect a tiny change in the dielectric constant, which is useful for investigating the nonlinear effect in active plasmonic components.

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Cited by 4 publications
(4 citation statements)
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“…A similar effect was observed recently in indium tin oxide nanorods supporting plasmons in the infrared [129]. There are interferometers in which refractive index modulation by a light pulse on a photo-refractive material induces a phase shift in one beam path changing the interference state and therefore the plasmon intensity [130][131][132][133]. This method can be used with magneto-optical materials [134].…”
Section: Modulation By External Lightsupporting
confidence: 69%
“…A similar effect was observed recently in indium tin oxide nanorods supporting plasmons in the infrared [129]. There are interferometers in which refractive index modulation by a light pulse on a photo-refractive material induces a phase shift in one beam path changing the interference state and therefore the plasmon intensity [130][131][132][133]. This method can be used with magneto-optical materials [134].…”
Section: Modulation By External Lightsupporting
confidence: 69%
“…Then, the surface was rinsed with ACT buffer for 5 min and reacted with mIgG dissolved in ACT buffer at a concentration of 50 μg/mL. The surface mass density of covalently immobilized mIgG was varied from Γ = 0 to 27 ng/mm 2 (as observed from respective changes in the thickness d h and refractive index n h (5)) by adjusting the reaction time between 0 and 60 min. Finally, the unreacted TFPS moieties were blocked by 20 min of incubating in a 1 M ETA solution, followed by rinsing with PBS for 10 min.…”
Section: Methodsmentioning
confidence: 99%
“…1 Fast and reversible tuning of surface plasmons is crucial to harness the potential of plasmonics in important areas such as signal processing, optical sensors, and biosensors. Up to now, the interfacing of metallic structures with dielectric materials for electro-optical, 2 thermo-optical, 3 magneto-optical, 4 photoinduced, 5 and electrochemical 6 -based modulating of refractive index was pursued for rapid tuning of surface plasmon resonance (SPR). However, these approaches typically allow for only weak refractive index changes (<10 –2 to 10 –3 ) 7 that are not sufficient to control SPR efficiently.…”
Section: Introductionmentioning
confidence: 99%
“…The sensitivity of plasmonic resonance to the refractive index of the dielectric surroundings affords us a convenient alternative to adjust the lasing wavelength through varying the refractive index. 22–24 Integrating plasmonic lattices within microfluidic channels and flowing liquid gain materials with different refractive indices has been proven to be very effective in dynamically modulating the output wavelength of plasmonic lasers. 25 Unfortunately, the reliance on liquid gain materials results in poor compactness and integrability of the devices, which restricts the practical applications in on-chip integration.…”
mentioning
confidence: 99%