2021
DOI: 10.1103/physrevresearch.3.033141
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Molecular polaritonics in dense mesoscopic disordered ensembles

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Cited by 28 publications
(26 citation statements)
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“…This observation could constitute the basis for an effective theory as developed in Ref. [38], which allows for the derivation of an effective unidirectional Markovian loss dynamics for the symmetric operator.…”
Section: This Is Based On the Orthonormality Conditionmentioning
confidence: 84%
“…This observation could constitute the basis for an effective theory as developed in Ref. [38], which allows for the derivation of an effective unidirectional Markovian loss dynamics for the symmetric operator.…”
Section: This Is Based On the Orthonormality Conditionmentioning
confidence: 84%
“… 142 Instead, the strongly delocalized electromagnetic field in the cavity opens up long-range interaction channels in a disordered ensemble of molecules. 143 This makes it highly challenging to infer photochemical properties of an ensemble of N molecules from the detailed study of a very restricted subset of it. To take into account the large number of emitters, one approach is to use strongly simplified molecular models, such as the Holstein model where each molecule is described by two displaced harmonic oscillators describing nuclear motion in the electronic ground and excited states.…”
Section: Theoretical Approaches and Challengesmentioning
confidence: 99%
“…z)P (E 1 )...P (E N ), (10) where P (E j ) is the disorder distribution function of E j . When evaluating G X,Y (z), N j=1 g 2 z+iEj → Π(z) in Eq.…”
Section: Thermodynamic Limit and Effective Hamiltonianmentioning
confidence: 99%
“…These states are denoted as 'dark states' and 'dark state reservoir' in the literature. Bright and dark states are theoretically understood accurately for homogeneous systems without disorder, while the nature of these states in the presence of disorder is still under debate [6][7][8][9][10][11][12][13][14][15][16][17]. * jianshu@mit.edu Specifically, disorder leads to a mixing of the dark states and the light field, such that they can contribute to spectroscopy and transport.…”
mentioning
confidence: 99%