Molybdenum-doped carbon nitride as an efficient heterogeneous catalyst for direct amination of nitroarenes with arylboronic acids

Li, Wen-Jing; Wang, Jun-Bo; Liu, Yu-Heng; Zhang, Mo; Zhang, Zhan-Hui

doi:10.1016/j.cclet.2024.110001

Chinese Chemical Letters

2024

DOI: 10.1016/j.cclet.2024.110001

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Molybdenum-doped carbon nitride as an efficient heterogeneous catalyst for direct amination of nitroarenes with arylboronic acids

Wen-Jing Li,

Jun-Bo Wang,

Yu-Heng Liu

et al.

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2024

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Cited by 3 publications

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Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Kang,

Yue,

et al. 2024

ACS Sustainable Chem. Eng.

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It is a great challenge to construct a green catalytic system for the reduction of nitro compounds to the corresponding amines under mild conditions. Due to the low energy of red light, it is challenging to develop photocatalytic selective reduction of nitroaromatics to aromatic amines driven by red light. A bimetallic porphyrin metal−organic framework (Bi-P(Co)MOF) was characterized by Fourier transform infrared spectroscopy, X-ray diffraction, transmission electron microscopy, scanning electron microscopy, and energy-dispersive X-ray techniques. The constructed photocatalyst Bi-PMOF-Co shows excellent catalytic activity for the conversion of nitro compounds to the corresponding amines in high to excellent yields with NaBH 4 as a mild reducing agent at room temperature under red light irradiation. Moreover, the photocatalytic protocol showed excellent functional group compatibility, and the recyclability of Bi-PMOF-Co was demonstrated by five-cycle tests.

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Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Kang,

Yue,

et al. 2024

ACS Sustainable Chem. Eng.

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Green and scalable synthesis of a dual-ligand Zn-MOF with unprecedented space–time yield in aqueous media and efficient CH₄/N₂ separation

Han,

Bai,

Zhao

et al. 2024

Green Chem.

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CdS/Mg–Fe layered double hydroxide: a versatile heterogeneous photocatalyst for the acylation of indoles with α-keto acids

Wang,

Yue,

et al. 2024

Green Chem.

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Molybdenum-doped carbon nitride as an efficient heterogeneous catalyst for direct amination of nitroarenes with arylboronic acids

Cited by 3 publications

References 45 publications

Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Green and scalable synthesis of a dual-ligand Zn-MOF with unprecedented space–time yield in aqueous media and efficient CH₄/N₂ separation

CdS/Mg–Fe layered double hydroxide: a versatile heterogeneous photocatalyst for the acylation of indoles with α-keto acids

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Molybdenum-doped carbon nitride as an efficient heterogeneous catalyst for direct amination of nitroarenes with arylboronic acids

Cited by 3 publications

References 45 publications

Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Bimetallic Porphyrin Metal–Organic Framework as Photocatalyst for Red-Light-Driven Selective Reduction of Nitroarenes to Aromatic Amines

Green and scalable synthesis of a dual-ligand Zn-MOF with unprecedented space–time yield in aqueous media and efficient CH4/N2 separation

CdS/Mg–Fe layered double hydroxide: a versatile heterogeneous photocatalyst for the acylation of indoles with α-keto acids

Contact Info

Product

Resources

About

Green and scalable synthesis of a dual-ligand Zn-MOF with unprecedented space–time yield in aqueous media and efficient CH₄/N₂ separation