Modern conceptual approach to geointerpretation and geoeducation emphasizes the holistic understanding of the environment and attends to linkages between various abiotic, biotic, and cultural components. In this paper, we highlight multiple relationships between Cenozoic volcanism and host sedimentary rocks, mainly sandstones of Cretaceous age, which can be explored in the context of geotourism and geoeducation in several Central European geoparks (Bohemian Paradise UNESCO Global Geopark, Land of Extinct Volcanoes Aspiring Geopark, Ralsko National Geopark) and their surroundings. These include the effects of magmatism on sandstones, with further consequences for landform development at different spatial scales, the origin of mineral resources, underpinning of biological diversity, and specific land use contrasts. Existing interpretation provisions are reviewed, and a three-tiered framework to show these different linkages is proposed. It is argued that different, but complementary themes can be addressed at the landscape, landform, and individual outcrop (geosite) level.