The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/admt.201900930.Metasurfaces, planar arrays composed of subwavelength engineered phase-shifting scatters, have been an emerging platform for advanced and functional control of electromagnetic (EM) waves by manipulating the local properties of amplitude, phase, and polarization of the reflected or transmitted waves. [1][2][3][4][5][6][7][8] The reliability and flexibility of wavefront manipulations by metasurfaces within subwavelength thickness then lead to many new physical effects and versatile applications, including anomalous light refraction, [4,5] invisibility cloak, [9] vortex beams, [10,11] and many other functional metadevices. [12][13][14][15][16][17][18][19] Nowadays, with the rapid development of modern wireless and optical technologies, increasing demands on high communication speed/quality, large data storage capacity are urgently required. The information capabilities of the metasurfaces can be