Neutron scattering shows that non-Fermi-liquid behavior of the heavy-fermion compound CeNi2Ge2 is brought about by the development of low-energy spin fluctuations with an energy scale of 0.6 meV. They appear around the antiferromagnetic wave vectors ( ). This unusual energy dependent structure of Imχ(Q, E) in Q space suggests that quasiparticle bands are important.PACS numbers: 75.30. Mb, 71.10.Hf, 71.27.+a Non-Fermi-liquid (NFL) behavior has been investigated in an increasing number of d-and f -electron systems in recent years [1,2]. In usual heavy-fermion systems, although strong correlation effects of f electrons bring about a mass renormalization m * /m by a factor of up to a few thousands, the systems remain in Fermi liquid (FL) states, which are typically observed as C/T = const and ρ − ρ 0 ∝ T 2 at low temperatures. The large mass enhancement originates from fluctuations of the spin degrees of freedom of the f electrons participating in the quasiparticles. When spin fluctuations are slowed down by certain mechanisms, the FL description breaks down, and NFL behavior appears as, for example, C/T ∝ ln(T 0 /T ) and ρ − ρ 0 ∝ T x with x < 2.A mechanism of NFL behavior is critical spin fluctuations near a quantum critical point (QCP), i.e., a zero-temperature magnetic phase transition, T N (or T C ) = 0 [2,3,4]. Observation of a QCP requires tuning of the competition between quenching of spin by the Kondo effect and interspin coupling by Ruderman-KittelKasuya-Yosida (RKKY) interactions using chemical substitutions, static pressures, or magnetic fields [5]. Recent experimental studies on critical behavior of CeCu 5.9 Au 0.1 [5,6] posed an intriguing theoretical question: Is the singularity described by the standard spin-fluctuation theories [3,4] or a locally critical quantum phase transition [2,7]? For chemically substituted systems, disorders inevitably affect singularities, ranging from perturbative effects to disorder-driven NFL behaviors [8]. Experiments using stoichiometric compounds showing NFL behavior without tuning, such as CeNi 2 Ge 2 [9] and YbRh 2 Si 2 [10], are thus expected to clarify the QCP or other mechanisms of NFL in the clean limit.CeNi 2 Ge 2 , which crystallizes in a body-centered tetragonal structure (see Fig. 1), is a paramagnetic heavy-fermion compound with enhanced C/T ≃ 350 mJ/K 2 mol [11]. It shows Kondo behavior with a temperature scale of T K ≃ 30 K [11] and has a metamagnetic behavior at H M ≃ 42 T [12]. For T < 5 K, i.e., well below T K , CeNi 2 Ge 2 exhibits NFL behavior with C/T ∝ ln(T 0 /T ) and ρ − ρ 0 ∝ T x , where 1 < x < 1.5 [9]. CeNi 2 Ge 2 also displays superconductivity near the QCP [13] which may be spin-fluctuation mediated [14].The NFL behavior has been thought to be caused by the spin fluctuations being slowed down by a QCP of an antiferromagnetic phase, which would be one of those observed in Pd, Rh, or Cu substituted compounds [15,16,17]. However, previous neutron-scattering experiments [18] on single crystalline CeNi 2 Ge 2 disagree with this simple interpreta...