2020
DOI: 10.1016/j.ijbiomac.2019.12.076
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Mussel-inspired cellulose-based adhesive with biocompatibility and strong mechanical strength via metal coordination

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Cited by 94 publications
(35 citation statements)
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“…Cytotoxicity evaluation is definitely indispensable when applying novel synthesized materials in human body. Right now, several published articles have reported the biocompatibility of mussel-inspired compounds in clinical application, including medical sealants [ 53 , 54 ], imaging agents [ 55 , 56 ], antifouling coatings [ 57 , 58 ] and adhesives [ 59 , 60 ], etc. In the current in vitro evaluation, a significant cytotoxicity of DMA was observed in the 50 ​μM concentration (47.96% cell viability) after 5-day incubation ( Fig.…”
Section: Discussionmentioning
confidence: 99%
“…Cytotoxicity evaluation is definitely indispensable when applying novel synthesized materials in human body. Right now, several published articles have reported the biocompatibility of mussel-inspired compounds in clinical application, including medical sealants [ 53 , 54 ], imaging agents [ 55 , 56 ], antifouling coatings [ 57 , 58 ] and adhesives [ 59 , 60 ], etc. In the current in vitro evaluation, a significant cytotoxicity of DMA was observed in the 50 ​μM concentration (47.96% cell viability) after 5-day incubation ( Fig.…”
Section: Discussionmentioning
confidence: 99%
“…Polysaccharide-based backbone materials for producing polyphenolic materials include chitosan [ 49 , 50 ], hyaluronic acid (HA) [ 51 , 52 , 53 ], alginate [ 54 , 55 ], collagen [ 56 ], and cellulose [ 57 ]. The majority of the grafting methods rely on EDC/NHS chemistry.…”
Section: Strategies To Design and Synthesize Polyphenolic Materials F...mentioning
confidence: 99%
“…The phenolic molecules for the EDC/NHS chemistry are chosen by considering the side-chain type. For example, a carboxyl group (–COOH) of polysaccharides was activated via EDC/NHS chemistry and became a conjugate by forming an amide bond with an amino group (–NH 2 ) from dopamine hydrochloride [ 49 , 50 , 51 , 52 , 53 , 54 , 55 , 56 , 57 , 82 ]. In contrast, amine-rich chitosan backbone was reacted with hydrocaffeic acid with a carboxylic acid group for the catechol functionalization [ 49 , 50 ].…”
Section: Strategies To Design and Synthesize Polyphenolic Materials F...mentioning
confidence: 99%
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“…Mussel-inspired adhesives are expected to serve as appropriate biological adhesives under wet conditions in clinical environments. Because of their excellent adhesion property, many researchers have investigated biomimetic catechol-functionalized natural/synthetic polymer-based tissue adhesives such as chitosan, alginic acid, hyaluronic acid, gelatin, silk fibroin, , cellulose, poly­(ethylene glycol), and poly­(acrylic acid). , When the catechol is oxidized to form the highly reactive quinone, the chemical cross-link is induced, which reacts with the nucleophile found on biological substrates, resulting in strong interfacial adhesion. , …”
Section: Introductionmentioning
confidence: 99%