Walnut green husk (WGH) is common agricultural by-product with high yield and serious pollution. The present study aimed to evaluate the impacts of solar drying (SD), pulsed vacuum drying (PVD), short and medium infrared radiation drying (SMIR), hot air drying based on temperature and humidity control (TH-HAD), and heat pump drying (HPD) on the drying characteristics, energy consumption, physicochemical properties, bioactive compounds content and antioxidant capacity of WGH. Drying characteristics and drying kinetics showed that artificial drying can significantly improve drying efficiency. Compared with SD, the drying time of PVD, SMIR, TH-HAD, and HPD were reduced by 63.57%, 78.68%, 66.28%, and 53.97%, respectively. Specific energy consumption analysis demonstrated that HPD showed the lowest specific energy consumption, 2.15 kW•h/kg. Hydration properties analysis revealed PVD had the best water holding capacity and HPD sample had the best water solubility index (43.44%). Structural analysis showed the cell wall structure of WGH was damaged by different drying methods. Overall, Among the five drying methods, HPD has lower energy consumption, less time, and maintains good antioxidant activity. HPD has good potential in the commercial-scale production of WGH.