Abstract:Rotationally-resolved infrared spectra of the bending modes of N 2 O-Ar and N 2 O-Kr van der Waals clusters have been studied in the region of the N 2 O ν 1 fundamental vibration (≈ 2224 cm −1 ), using a tunable quantum cascade laser source to probe complexes generated in pulsed supersonic jet expansion. The assigned vibrational transitions are hot bands (1, 1 1 , 0)← (0, 1 1 , 0) observed under supersonic conditions. In the presence of Argon/Krypton atom, the doubly-degenerate ν 2 bending mode of the N 2 O mo… Show more
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