Na-ion dynamics in the solid solution NaxCa1−xCr2O4 studied by muon spin rotation and neutron diffraction

Nocerino, Elisabetta; Forslund, Ola Kenji; Sakurai, Hiroya; Matsubara, Nami; Zubayer, Anton; Mazza, Federico; Cottrell, Stephen; Koda, Akihiro; Watanabe, Isao; Hoshikawa, Akinori; Saito, Takashi; Sugiyama, Jun; Sassa, Yasmine; Månsson, Martin

doi:10.1039/d3se01097j

Sustainable Energy Fuels

2024

DOI: 10.1039/d3se01097j

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Na-ion dynamics in the solid solution Na_xCa_1−xCr₂O₄ studied by muon spin rotation and neutron diffraction

Elisabetta Nocerino,

Ola Kenji Forslund,

Hiroya Sakurai

et al.

Abstract: In this work we present systematic set of measurements carried out by muon spin rotation/relaxation (μ+SR) and neutron powder diffraction (NPD) on the solid solution NaxCa1- xCr2O4. This study investigates...

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Cr-Cr distance and magnetism in the phase diagram of triangular lattice antiferromagnets: A systematic comparative study

Nocerino,

Sugiyama,

Forslund

et al. 2024

Phys. Rev. Materials

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In this study, we investigate the influence of Cr-Cr distances on the magnetic properties of triangular lattice antiferromagnets through the lens of the recently synthesized Cr compounds LiCrSe2, LiCrTe2, and NaCrTe2. Our comprehensive analysis integrates existing magnetic structure data and new insights from muon spin rotation measurements, revealing a striking mutual influence between strongly correlated electrons and structural degrees of freedom in systems possessing very different magnetic properties despite having the same crystal symmetry. In particular, we delineate how Cr-Cr distances specifically dictate the magnetic behaviors of the triangular lattice antiferromagnets LiCrSe2, LiCrTe2, and NaCrTe2. By crafting phase diagrams based on these distances, we establish a clear correlation between the structural parameters and the magnetic ground states of these materials together with a wide variety of trivalent Cr triangular lattice layered magnets. Our analysis uncovers a transition range for in-plane and out-of-plane Cr-Cr distances that demarcates distinct magnetic behaviors, highlighting the nuanced role of lattice geometry in the spin-lattice interaction and electron correlation dynamics. Published by the American Physical Society 2024

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Cr-Cr distance and magnetism in the phase diagram of triangular lattice antiferromagnets: A systematic comparative study

Nocerino,

Sugiyama,

Forslund

et al. 2024

Phys. Rev. Materials

View full text Add to dashboard Cite

show abstract

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Na-ion dynamics in the solid solution Na_xCa_1−xCr₂O₄ studied by muon spin rotation and neutron diffraction

Abstract: In this work we present systematic set of measurements carried out by muon spin rotation/relaxation (μ+SR) and neutron powder diffraction (NPD) on the solid solution NaxCa1- xCr2O4. This study investigates...

Cited by 1 publication

References 77 publications

Cr-Cr distance and magnetism in the phase diagram of triangular lattice antiferromagnets: A systematic comparative study

Cr-Cr distance and magnetism in the phase diagram of triangular lattice antiferromagnets: A systematic comparative study

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