2021
DOI: 10.1038/s41467-021-21862-5
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Nano-imaging photoresponse in a moiré unit cell of minimally twisted bilayer graphene

Abstract: Graphene-based moiré superlattices have recently emerged as a unique class of tuneable solid-state systems that exhibit significant optoelectronic activity. Local probing at length scales of the superlattice should provide deeper insight into the microscopic mechanisms of photoresponse and the exact role of the moiré lattice. Here, we employ a nanoscale probe to study photoresponse within a single moiré unit cell of minimally twisted bilayer graphene. Our measurements reveal a spatially rich photoresponse, who… Show more

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Cited by 55 publications
(38 citation statements)
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“…Graphene, an amazing carbon-related two-dimensional nanomaterial with distinct electrical, thermal, and mechanical properties, has become extremely popular in biomedical field since its discovery in 2004 [73]. This newly proposed material possesses large surface area, great biocompatibility, good stability, distinctive thermal and optical properties, and superb conductivity [74].…”
Section: Graphene-based Nanomaterialsmentioning
confidence: 99%
“…Graphene, an amazing carbon-related two-dimensional nanomaterial with distinct electrical, thermal, and mechanical properties, has become extremely popular in biomedical field since its discovery in 2004 [73]. This newly proposed material possesses large surface area, great biocompatibility, good stability, distinctive thermal and optical properties, and superb conductivity [74].…”
Section: Graphene-based Nanomaterialsmentioning
confidence: 99%
“…Despite extensive studies on twisted bilayer graphene, based on transport and scanning techniques, and several interesting theoretical predictions [256][257][258][259][260] , a complete study of its optical properties 261,262 , in particular at low temperatures, where the symmetry-broken states arise is still lacking. In this context, nanophotonics probes like s-SNOM 261,262 and spectroscopy are ideal candidates since they are able to conjugate high spatial resolution (down to ≈ 10nm), with energies that are matching the expected optical features, often in the mid-Infrared or Terahertz (THz) frequency ranges (cf. Figure 7a-b).…”
Section: Moiré Systemsmentioning
confidence: 99%
“…The curved arrows indicate the light impinging on the tip (coming from the laser) as well as the scattered light (going to the detector). Adapted from ref262 . b: 2D plots of the energy loss function L(q, ω) at θ = 1.05°.…”
mentioning
confidence: 99%
“…b. Indirect lattice matching between materials with very different lattice constants for epitaxial integration c. Wafer bonding, using a thin film of amorphous material d. polycrystaline integration on a substrate e. integration based on 2D materials, wher ethe weak out of plane bonding allows different materials to couple without lattice matching f. recent demonstration of integration of 2D materials with optoelectronically active graphene, from reference [179] sible in this platform [192,193]. Other materials, such as black phosphorous [194] and platinum diselenide [195] show potential for detection of infrared light.…”
Section: D Materialsmentioning
confidence: 99%