Giant magnetoimpedance effect in ultrasoft FeAlSiBCuNb nanocomposites for sensor applications J. Appl. Phys. 98, 014316 (2005); 10.1063/1.1953864 Valve behavior of giant magnetoimpedance in field-annealed Co 70 Fe 5 Si 15 Nb 2.2 Cu 0.8 B 7 amorphous ribbon nanocomposite materials consisting of nanocrystalline phase in an amorphous matrix were obtained by heat-treatment of their precursor amorphous ribbons. The influence of structural modifications induced during the heat-treatment on soft magnetic properties and magnetoimpedance (MI) effect have been studied. The structural investigations on both these ribbons revealed the presence of two phases, fine grained Fe 3 Si phase and a residual amorphous phase on heat-treatment. The maximum MI ratio obtained in the present study is 95% at f ¼ 4 MHz, for the optimized heat-treated Fe 77.2 Si 11.2 Cu 0.8 Nb 3.3 B 7.5 ribbon. This is ascribed to the increase in magnetic permeability and decrease in coercive force and intrinsic resistivity. Moreover, a maximum magnetic field sensitivity (n) of 8.3%/Oe at f ¼ 2.5 MHz is obtained, for the optimized nanocrystalline Fe 73.5 Si 13.5 Cu 1 Nb 3 B 9 ribbon. This suggests that tailoring of the nanocrystalline microstructures induced by optimum heat-treatment conditions can result in obtaining excellent combinations of the magnetic permeability and resistivity. Our results indicate that these Fe-based nanocrystalline materials can be ideally used for low magnetic field and high frequency sensor applications.