Nature of the<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi></mml:math>Phase in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msub><mml:mrow><mml:mi>CeCu</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mi>Si</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math>

Stockert, O.; Faulhaber, E.; Zwicknagl, Gertrud; Stüßer, N.; Jeevan, H. S.; Deppe, M.; Borth, R.; Küchler, R.; Loewenhaupt, M.; Geibel, C.; Steglich, F.

doi:10.1103/physrevlett.92.136401

Cited by 130 publications

(131 citation statements)

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“…* Corresponding author: Dmytro.Inosov@tu-dresden. de A handful of earlier works on magnetic heavy-fermion metals, where conduction electrons are involved in the formation of magnetic order, suggest that the low-energy dynamic spin susceptibility χ(ω, Q), measured with diffuse neutron scattering, provides direct information about the nesting vectors [7][8][9][10][11][12][13][14][15][16]. Due to the bulk sensitivity of neutron scattering, it therefore serves as a complementary method for probing the 3D electronic structure.…”

Section: Introductionmentioning

confidence: 99%

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
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We investigate the doping-induced changes in the electronic structure of CeB 6 on a series of substituted Ce 1−x R x B 6 samples (R = La, Nd) using diffuse neutron scattering. We observe a redistribution of magnetic spectral weight across the Brillouin zone, which we associate with the changes in the Fermi-surface nesting properties related to the modified charge carrier concentration. In particular, a strong diffuse peak at the corner of the Brillouin zone (R point), which coincides with the propagation vector of the elusive antiferroquadrupolar (AFQ) order in CeB 6 , is rapidly suppressed by both La and Nd doping, like the AFQ order itself. The corresponding spectral weight is transferred to the X (00 1 2 ) point, ultimately stabilizing a long-range AFM order at this wave vector at the Nd-rich side of the phase diagram. At an intermediate Nd concentration, a broad diffuse peak with multiple local maxima of intensity is observed around the X point, evidencing itinerant frustration that gives rise to multiple ordered phases for which Ce 1−x Nd x B 6 is known. On the La-rich side of the phase diagram, however, dilution of the magnetic moments prevents the formation of a similar (00 1 2 )-type order despite the presence of nesting. Our results demonstrate how diffuse neutron scattering can be used to probe the nesting vectors in complex f-electron systems directly, without reference to the single-particle band structure, and emphasize the role of Fermi surface geometry in stabilizing magnetic order in rare-earth hexaborides.

show abstract

Section: Introductionmentioning

confidence: 99%

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
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“…Much of the physics of the phase diagram is driven by a quantum critical point, which separates long-range ordered ground states from those in which the local moments have fully hybridized with the conduction electrons to form itinerant states with large effective masses and large Fermi surfaces (5). In several materials quantum critical fluctuations give rise to anomalous non-Fermi liquid behavior in various bulk transport and thermodynamic quantities (6)(7)(8).…”

mentioning

confidence: 99%

Long range order and two-fluid behavior in heavy electron materials

Shirer

Shockley

Dioguardi

et al. 2012

Proc. Natl. Acad. Sci. U.S.A.

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The heavy electron Kondo liquid is an emergent state of condensed matter that displays universal behavior independent of material details. Properties of the heavy electron liquid are best probed by NMR Knight shift measurements, which provide a direct measure of the behavior of the heavy electron liquid that emerges below the Kondo lattice coherence temperature as the lattice of local moments hybridizes with the background conduction electrons. Because the transfer of spectral weight between the localized and itinerant electronic degrees of freedom is gradual, the Kondo liquid typically coexists with the local moment component until the material orders at low temperatures. The two-fluid formula captures this behavior in a broad range of materials in the paramagnetic state. In order to investigate two-fluid behavior and the onset and physical origin of different long range ordered ground states in heavy electron materials, we have extended Knight shift measurements to URu 2 Si 2 , CeIrIn 5 , and CeRhIn 5 . In CeRhIn 5 we find that the antiferromagnetic order is preceded by a relocalization of the Kondo liquid, providing independent evidence for a local moment origin of antiferromagnetism. In URu 2 Si 2 the hidden order is shown to emerge directly from the Kondo liquid and so is not associated with local moment physics. Our results imply that the nature of the ground state is strongly coupled with the hybridization in the Kondo lattice in agreement with phase diagram proposed by Yang and Pines.nuclear magnetic resonance | heavy fermion | hyperfine couplings C ompetition between different energy scales gives rise to a rich spectrum of emergent ground states in strongly correlated electron materials. In the heavy fermion compounds, a lattice of nearly localized f electrons interacts with a sea of conduction electrons, and depending on the magnitude of this interaction different types of long-range order may develop at low temperatures (1). The Kondo lattice model strives to capture the essential physics of heavy fermion materials by considering the various magnetic interactions between the conduction electron spins, S c , and the local moment spins, S f (2). Different ground states can emerge depending on the relative strengths of the interaction, J, between S c and S f and the intersite interaction, J f f , between the S f spins (3, 4). Much of the physics of the phase diagram is driven by a quantum critical point, which separates long-range ordered ground states from those in which the local moments have fully hybridized with the conduction electrons to form itinerant states with large effective masses and large Fermi surfaces (5). In several materials quantum critical fluctuations give rise to anomalous non-Fermi liquid behavior in various bulk transport and thermodynamic quantities (6-8).In recent years, evidence has emerged that in the high temperature disordered phase the electronic degrees of freedom simultaneously exhibit both itinerant and localized behavior (9). Below a temperature T Ã that marks the onset...

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“…6,7 The development of a new predictive "standard model" for heavy electron materials -a phenomenological two-fluid description, in which two coexisting electronic fluids emerge below a collective hybridization temperature T * , has changed our physical picture of how this dichotomy manifests itself.…”

mentioning

confidence: 99%

Kondo liquid emergence and relocalization in the approach to antiferromagnetic ordering in CePt2In7

et al. 2011

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Nature of theAPhase inCeCu2Si2

Cited by 130 publications

References 15 publications

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
View full text Add to dashboard Cite

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
View full text Add to dashboard Cite

Long range order and two-fluid behavior in heavy electron materials

Kondo liquid emergence and relocalization in the approach to antiferromagnetic ordering in CePt2In7

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Nature of theAPhase inCeCu2Si2

Cited by 130 publications

References 15 publications

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and Nikitin1, Portnichenko2, Dukhnenko3 et al. 2018Phys. Rev. B123160View full textAdd to dashboardCite

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and Nikitin1, Portnichenko2, Dukhnenko3 et al. 2018Phys. Rev. B123160View full textAdd to dashboardCite

Long range order and two-fluid behavior in heavy electron materials

Kondo liquid emergence and relocalization in the approach to antiferromagnetic ordering in CePt2In7

Contact Info

Product

Resources

About

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
View full text Add to dashboard Cite

Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides Ce1−xLaxB6 and
Nikitin
¹
,
Portnichenko
²
,
Dukhnenko
³

et al. 2018
Phys. Rev. B
12
3
16
0
View full text Add to dashboard Cite