Lithography, the
transfer of patterns to a film or substrate, is
the basis by which many modern technological devices and components
are produced. However, established lithographic approaches generally
use complex techniques, expensive equipment, and advanced materials.
Here, we introduce a water-based microcontact printing method using
silk that is simple, inexpensive, ecofriendly, and recyclable. Whereas
the traditional microcontact printing technique facilitates only negative
lithography, the synergetic interaction of the silk, water, and common
chemicals in our technique enables both positive and negative patterning
using a single stamp. Among diverse application possibilities, we
exemplify a proof of concept of the method through optimizing its
metal lift-off process and demonstrate the fabrication of electromagnetic
metamaterial elements on both solid and flexible substrates. The results
indicate that the method demonstrated herein is universally applicable
to device production and technology development.