Extraordinary properties of nonlinear optical propagation processes in double-domain positive/negative index metamaterials are reviewed. These processes enable coherent energy exchange between ordinary and backward electromagnetic waves, which allows huge increase of frequency-conversion efficiency at second harmonic generation, three-wave mixing and optical parametric amplification. Striking contrasts with properties of the counterparts in ordinary materials are outlined. Particularly, exotic features arise for amplification and generation of counter-propagating short pulses. Novel class of materials, which enable such processes through electromagnetic waves with negative group velocity, are proposed. The possibility to mimic such processes in readily available crystals that support elastic backward waves (optical phonons) is shown. The concepts of unique photonic devices such as data processing chips, tunable nonlinear-optical mirrors, filters, switches and sensors are discussed.
IntroductionOptical negative-index materials (NIMs) form a class of electromagnetic media that promise revolutionary breakthroughs in photonics. The possibilities of such breakthroughs originate from backwardness, the exotic property that electromagnetic waves (EMWs) acquire in NIMs. Unlike ordinary positive-index materials, the energy flow, S, and the wave-vector, k, become counter-directed in NIMs that determines their unique linear and nonlinear optical (NLO) propagation properties. The appearance of backward electromagnetic waves (BEMW) can be explained as follows. The direction of the wave-vector k with respect to the energy flow S