Specific satellites with ultralong wings play a crucial role in many fields. However, external disturbance and self-rotation could result in undesired vibrations of the flexible wings, which affect the normal operation of the satellites. In severe cases, the satellites would be damaged. Therefore, it is imperative to conduct vibration suppression for these flexible structures. Utilizing fuzzy-proportional integral derivative control and deep reinforcement learning (DRL), two active control methods are proposed in this article to rapidly suppress the vibration of flexible structures with quite small controllable force based on a cable-driven parallel robot. Inspired by the output law of DRL, a new control method named Tang and Sun control is innovatively presented based on the Lyapunov theory. To verify the effectiveness of these three control methods, three groups of simulations with different initial disturbances are implemented for each method. Besides, to enhance the contrast, a passive pretightening scheme is also tested. First, the dynamic model of the cable-driven parallel robot which comprises four cables and a flexible structure is established using the finite element method. Then, the dynamic behavior of the model under the controllable cable force is analyzed by the Newmark-ß method. Finally, these control methods are implemented by numerical simulations to evaluate their performance, and the results are satisfactory, which validates the controllers’ ability to suppress vibrations.