“…In our simulation, the nonlinearity of the polystyrene electronic system was represented by a two‐level electronic system, as described in Section 2. Theoretically, it is easy to prove that when the electronic system is pumped by a time‐independent power, it corresponds to a Kerr‐like nonlinear material owing to the variation in the population difference
,
21 where
and
are the populations at the lower level with and without pumping, respectively, and
is the population at the upper level. Here, we set
, while the lifetime of electrons on the upper level is set as
s, which is a typical value for intraband electronic processes.…”