Nondestructive determination of isotopic abundance using multi-energy nuclear resonance fluorescence driven by laser Compton scattering source

Abstract

We report on the quantitative nondestructive analysis of the natural isotopic abundances of hafnium and tungsten elements using nuclear resonance fluorescence. Metallic samples of hafnium and tungsten were irradiated to six quasi-monochromatic γ-ray beams generated by laser Compton scattering in the energy range of 2.4–3.2 MeV. Multiple nuclei were simultaneously excited at each of the six γ-ray beam energies. A high-purity germanium detector array detected deexcitations of the nuclei. In total, 51 transitions were unprecedentedly employed to estimate the isotopic abundances of heavy elements nondestructively. The estimated abundances of three hafnium isotopes and three tungsten isotopes are consistent with standard known natural abundances within the experimental uncertainties. The deviation from the standard values ranges from 0.18% to 1.36%.