“…Organic nonlinear optical (NLO) materials have attracted considerable attention in recent years due to their intriguing properties, such as structural exibility, large p-conjugated systems, and biocompatibility, and are highly promising for applications in all-optical switching, optical limiting, bioimaging, and so on. [1][2][3][4][5] It is well known that the NLO response of conjugated organic materials is closely related to the structure of the molecule, such as the size of the p-conjugated system and the introduction of electron donor and electron acceptor. [6][7][8][9][10] Hence, designing novel organic chromophores exhibiting superior NLO response is of great scientic and technological interest not only for shedding light on the nonlinear light-matter interaction but also for the development of novel photonic devices.…”