2019
DOI: 10.1364/optica.6.000878
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Nonlinear optics with full three-dimensional illumination

Abstract: We investigate the nonlinear optical process of third-harmonic generation in the thus far unexplored regime of focusing the pump light from a full solid angle, where the nonlinear process is dominantly driven by a standing dipole-wave. We elucidate the influence of the focal volume and the pump intensity on the number of frequency-tripled photons by varying the solid angle from which the pump light is focused, finding good agreement between the experiments and numerical calculations. As a consequence of focusi… Show more

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Cited by 9 publications
(13 citation statements)
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“…In the low-frequency regime, the nonparaxial light propagation cannot be simply mapped to a Schrödinger-type wave equation. For example, a recent study 56 revealed that a tightly focused nonparaxial light beam can enhance nonlinear optical interactions. However, no attempt has been done to explore the topological properties of nonparaxial light.…”
Section: Introductionmentioning
confidence: 99%
“…In the low-frequency regime, the nonparaxial light propagation cannot be simply mapped to a Schrödinger-type wave equation. For example, a recent study 56 revealed that a tightly focused nonparaxial light beam can enhance nonlinear optical interactions. However, no attempt has been done to explore the topological properties of nonparaxial light.…”
Section: Introductionmentioning
confidence: 99%
“…However, the paraxial approximation is not always strictly satisfied in waveguide systems, and in fact nonparaxial light is quite ubiquitous in natural photonic systems, such as spin-orbit interaction of nonparaxial light [21,22], nonparaxial Airy beams [23][24][25][26][27][28] and other nonparaxial accelerating beams [29][30][31], etc. Recently, nonparaxiality has attracted growing interests, which has been shown to play an important role in third-harmonic generation [32] and asymmetric topological pumping [33]. Nevertheless, the study of nonparaxial wave propagation and related phenomena is still in its infancy, and it still remains elusive how nonparaxiality can benefit the field of photonics.…”
Section: Introductionmentioning
confidence: 99%
“…The resulting focal spot has a size which is on a par with or better than that of high quality lens objectives [2,3]. Parabolic mirrors have found multiple applications in confocal microscopy [4], cryostat based single molecule spectroscopy [5], scanning optical near-field microscopy [6], Raman microscopy [7], solar cells [8], light-emitting diodes [9], nonlinear optics [10]. Recently, deep parabolic mirrors gained attention in quantum optics because of their efficient focusing, ability of trapping individual quantum emitters, and of extracting a collimated beam of single photons [11,12].…”
Section: Introductionmentioning
confidence: 99%