2004
DOI: 10.1002/app.20537
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Nonlinear stress relaxation in palladium(II) complexes with triblock copolymers of styrene and butadiene

Abstract: Above 200% strain, the mechanical response of triblock copolymers which contain styrene and butadiene is modified significantly by complexation with dichlorobis(acetonitrile)palladium(II). This pseudosquare-planar transition metal salt forms -complexes with, and catalyzes the dimerization of, alkene groups in the main chain and the side group of Kraton's butadiene midblock. Between 10 and 100% strain, the plastic flow regime is similar for undiluted Kraton™ and its Pd 2ϩ complexes, but the level of engineering… Show more

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