The generation of surface plasmon–polariton (SPP) pulses on the first and second harmonics of a carrier wave is considered at the boundary of a uniaxial crystal and non-magnetic metal. The SPP pulses on the first and second harmonics can arise in the forms of bright and dark solitons, or as cnoidal waves, in accordance with the velocity synchronism of the SPP pulses. The variation of the interaction efficiency and the changes of forms of the SPP pulses due to the exact or non-exact synchronism of their velocities have been investigated. It is shown that the selection of pairs of the crystal and metal allows changes in the forms of the SPP pulses.