This research study addresses the issues with additive manufacturing of high abrasive concentration as well as highly affordable resin-bond grinding wheels. High-concentration resin bond grinding wheels are high-demand cutting tools that provide high-efficiency grinding operation for a broad range of ferrous and nonferrous metals. Adding a high concentration of abrasive grains into the blend while using high-temperature acrylic resins as a bond material has encountered some difficulties during digital light processing (DLP), such as insufficient flow of material resulting from the high inherent viscosity of the pure resin and less printability due to their dark color, which become worse by adding a high volume of abrasive grains. An engineered bond material achieved through the mechanical alloying of acrylate photopolymers with tailored properties has been discovered during this research study, taking advantage of reduced price, excellent grinding performance, and high grain concentration. The experimental grinding operations comprising medium and high material removal rates were carried out to prove the supreme properties of the SiC- and diamond-printed grinding wheels toward having high accuracy besides a high-quality finished surface. Mechanical characterization including tensile test and grinding performance examination comprising tool wear, cutting force, surface quality, and surface integrity were conducted on the printed and ground parts. The results showed that integrating 14.6 Wt% of Resin A (with higher thermal resistance and viscosity) into the wheel’s composition could contribute to the fabrication of a high-performance grinding wheel, besides having a reliable, fast, and feasible printing process. Furthermore, On-machine and out-of-machine measurements on the ground surface signified that the composition with the highest Resin B concentration (GW-H) offered up to 2 times higher mechanical properties, 33–50% lower grinding forces, 25–50% improved surface qualities, 2–3 times extended tool life span, and less interval dressing operation compared to the grinding wheel containing the lowest Resin B concentration (GW-L).