Observation of recollision-based high-harmonic generation in liquid isopropanol and the role of electron scattering

Alexander, Oliver; Barnard, Jonathan C. T.; Larsen, Esben W.; Avni, Timur; Jarosch, Sebastian; Ferchaud, Clément; Gregory, Andrew; Parker, Susan; Galinis, Gediminas; Tofful, Alexandra; Garratt, Douglas; Matthews, Mary R.; Marangos, Jonathan P.

doi:10.1103/physrevresearch.5.043030

Phys. Rev. Research

2023

DOI: 10.1103/physrevresearch.5.043030

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Observation of recollision-based high-harmonic generation in liquid isopropanol and the role of electron scattering

Oliver Alexander,

Jonathan C. T. Barnard,

Esben W. Larsen

et al.

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Cited by 5 publications

(1 citation statement)

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“…The optical control of attosecond pulses continues to increase, including the use of structured light, 58 tailored polarizations, 59 chiral states of light, 60 attosecond frequency combs based on femtosecond enhancement cavities, 61 and detailed control of the HHG wavefronts. 62 Attosecond science also continues to expand the range of systems it can study, from HHG in solids 63 to liquids 64 and nanostructures. 65 Its growth has also made it possible to build fertile interfaces with other branches of physics, including quantum optics, 66 and quantum information processing, 67 which hold substantial promise of innovation for this youngbut now matureand dynamic discipline.…”

mentioning

confidence: 99%

Shining the shortest flashes of light on the secret life of electrons

Khokhlova,

Pisanty,

Zaïr

2023

Adv. Photon.

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mentioning

confidence: 99%

Shining the shortest flashes of light on the secret life of electrons

Khokhlova,

Pisanty,

Zaïr

2023

Adv. Photon.

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Liquid crystal-based temperature-controlled recirculating flat jet system

Murillo-Sánchez,

Copete-Plazas,

Bürkle

et al. 2024

Review of Scientific Instruments

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In this paper, the design and implementation of a temperature-controlled recirculating flat jet system for liquid crystals (LCs)-based experiments are presented. In these experiments, the target liquid is usually exposed to medium to high laser fluences, possibly resonant with specific excitation, thus resulting in a change of local temperature and sudden degradation. To overcome this problem, each laser pulse must interact with a new volume of liquid, preferably with flat surfaces, while avoiding the use of substrates. A well-established solution consists of impinging two identical laminar jets that force the liquid into a radial expansion perpendicular to the plane formed by the jets, resulting in a consecutive chain of flat sheets bound by thick rims. In this context, LCs pose several challenges considering their viscosity, non-Newtonian behavior, and mesophase nature. Here, a precise control of temperature, thus mesophase, and pressure is demonstrated enabling the use of LCs in an impinging jet system. In particular, the system presented here delivers stable fluid chains of different sizes and thicknesses. The viscosity and non-Newtonian behavior of the LCs have a significant impact on the thickness of the chains as a function of the nozzle inner diameter, impinging angle, and radial distance from the impinging point. The flow rate, on the other hand, primarily affects the width and length of the liquid sheet.

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Linking high-order harmonic generation and radial distribution function in liquids

Li,

Chen,

Ding

et al. 2024

Phys. Rev. A

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Observation of recollision-based high-harmonic generation in liquid isopropanol and the role of electron scattering

Cited by 5 publications

References 57 publications

Shining the shortest flashes of light on the secret life of electrons

Shining the shortest flashes of light on the secret life of electrons

Liquid crystal-based temperature-controlled recirculating flat jet system

Linking high-order harmonic generation and radial distribution function in liquids

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