Attempts to apply quantum collapse theories to Cosmology and cosmic inflation are reviewed. These attempts are motivated by the fact that the theory of cosmological perturbations of quantummechanical origin suffers from the single outcome problem, which is a modern incarnation of the quantum measurement problem, and that collapse models can provide a solution to these issues. Since inflationary predictions can be very accurately tested by cosmological data, this also leads to constraints on collapse models. These constraints are derived in the case of Continuous Spontaneous Localization (CSL) and are shown to be of unprecedented efficiency.