Although air quality in the United States improved remarkably in the past decades, ground-level ozone (O3) 20 rises often in exceedance of the national ambient air quality standard in nonattainment areas, including the Long Island Sound (LIS) and its surrounding areas. Accurate prediction of high ozone episodes is needed to assist government agencies and the public in mitigating harmful effects of air pollution. In this study, we have developed a suite of potential forecast improvements, including dynamic boundary conditions, rapid emission refresh and chemical data assimilation, in a 3 km resolution Community Multi-scale Air Quality (CMAQ) modeling system. The purpose is to evaluate and assess 25 the effectiveness of these forecasting techniques, individually or in combination, in improving forecast guidance for two major air pollutants: surface O3 and nitrogen dioxide (NO2). Experiments were conducted for a high O3 episode (August 28-29, 2018) during the Long Island Sound Tropospheric Ozone Study (LISTOS) field campaign, which provides abundant observations for evaluating model performance. The results show that these forecast system updates are useful in enhancing the capability of the forecasting model with varying effectiveness for different pollutants. For O3 prediction, 30 the most significant improvement comes from the dynamic boundary conditions derived from NOAA National Air Quality Forecast Capability (NAQFC), which increases the correlation coefficient (R) from 0.81 to 0.93 and reduces the Root Mean Square Error (RMSE) from 14.97 ppbv to 8.22 ppbv, compared to that with the static boundary conditions.The NO2 from all high-resolution simulations outperforms that from the operational 12 km NAQFC simulation, highlighting the importance of spatially resolved emission and meteorology inputs for the prediction of short-lived 35 pollutants. The effectiveness of improved initial concentrations through optimal interpolation (OI) is shown to be high in urban areas with high emission density. The influence of OI adjustment, however, is maintained for a longer period in rural areas where emissions and chemical transformation make a smaller contribution to the O3 budget than that in high emission areas. Following the assessment of individual forecast system updates, the forecasting system is configured with dynamic boundary conditions, optimal interpolation of initial concentrations, and emission adjustment, to simulate the 40