2019
DOI: 10.1021/acs.accounts.9b00002
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On Controllability and Applicability of Surface Molecular Self-Assemblies

Abstract: Conspectus Molecular self-assembly (MSA) refers to spontaneous arrangement of molecular building blocks into ordered structures governed by weak interactions. Due to its high versatility and reversibility, MSA has been widely employed as a robust bottom-up approach to fabricating low-dimensional functional nanostructures, which are used in various applications in nanoscience and technology. To date, tremendous effort has been devoted to constructing various MSAs at surfaces, ranging from self-assembled monolay… Show more

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Cited by 64 publications
(71 citation statements)
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“…Successful design of chemical systems with targeted functions/properties relies heavily on novel approaches for governing the molecular assembly. Alongside non‐covalent interactions, reversible covalent bonds have been frequently utilized in the design and synthesis of numerous functional molecules, with applications in materials chemistry, catalysis, recognition, sensing, cargo delivery, as well as flourished in the field of dynamic combinatorial chemistry . Moreover, due to their dynamic nature, reversible covalent bonds facilitate the high‐yielding synthesis of mechanically interlocked molecules such as catenanes, rotaxanes, and knots, representing important components of molecular machines .…”
Section: Figurementioning
confidence: 99%
“…Successful design of chemical systems with targeted functions/properties relies heavily on novel approaches for governing the molecular assembly. Alongside non‐covalent interactions, reversible covalent bonds have been frequently utilized in the design and synthesis of numerous functional molecules, with applications in materials chemistry, catalysis, recognition, sensing, cargo delivery, as well as flourished in the field of dynamic combinatorial chemistry . Moreover, due to their dynamic nature, reversible covalent bonds facilitate the high‐yielding synthesis of mechanically interlocked molecules such as catenanes, rotaxanes, and knots, representing important components of molecular machines .…”
Section: Figurementioning
confidence: 99%
“…Successful design of chemical systems with targeted functions/properties relies heavily on novel approaches for governing the molecular assembly. Alongside non‐covalent interactions, reversible covalent bonds have been frequently utilized in the design and synthesis of numerous functional molecules, with applications in materials chemistry, catalysis, recognition, sensing, cargo delivery, as well as flourished in the field of dynamic combinatorial chemistry . Moreover, due to their dynamic nature, reversible covalent bonds facilitate the high‐yielding synthesis of mechanically interlocked molecules such as catenanes, rotaxanes, and knots, representing important components of molecular machines .…”
Section: Figurementioning
confidence: 99%
“…This empirical relation describes most chemical reactions well. 2 Yet though the equation itself is simple, its chemical meaning is elusive. This is especially true for the nefarious pre-exponential factor.…”
Section: Introductionmentioning
confidence: 99%