This paper is an attempt to establish the existence and multiplicity results of nontrivial solutions to singular systems with sign-changing weight, nonlinear singularities, and critical exponent. By using variational methods, the Nehari manifold, and under sufficient conditions on the parameter η which represent some physical meanings, we prove some existing results by researching the critical points as the minimizers of the energy functional associated with the proposed problem (2) on the constraint defined by the Nehari manifold, which are solutions of our system, under some sufficient conditions on the parameters α, β, μ, and η. To the best of our knowledge, this paper is one of the first contributions to the study of singular systems with sign-changing weight, nonlinear singularities, and critical exponent.