Bimetal sheets have superior properties as they combine different materials with different characteristics. Producing bimetal parts using a single-point incremental forming process (SPIF) has increased recently with the development of industrial requirements. Such types of sheets have multiple functions that are not applicable in the case of monolithic sheets. In this study, the correlation between the operating variables, the maximum forming angle, and the surface roughness is established based on the ensemble learning using gradient boosting regression tree (GBRT). In order to obtain the dataset for the machine learning, a series of experiments with continuous variable angle pyramid shape were carried out based on D-Optimal design. This design is created based on numerical variables (i.e., tool diameter, step size, and feed rate) and categorical variable (i.e., layer arrangement). The grid search cross-validation (CV) method was used to determine the optimum GBRT parameters prior to model training. After the parameter tuning and model selection, the model with a better generalization performance is obtained. The reliability of the predictive models is confirmed by the testing samples. Furthermore, the microstructure of the aluminum/stainless steel (Al/SUS) bimetal sheet is analyzed under different levels of operating parameters and layer arrangements. The microstructure results reveal that severe cracks are attained in the case of a small tool diameter while a clear refinement is observed when a high tool diameter value with small step down is used for both Al and SUS layers. different materials that have different characteristics, this strengthens the conductivity, corrosion resistance, and the yield strength of the combined sheet. The application of such processes to produce the desired composite parts combines the characteristics of both the forming process and the parent materials to enhance the quality and the formability of the low formable materials and reduce the cost and the weight of manufactured parts.The SPIF of composite sheets has generated considerable recent research interest. In the study of Al-Ghamdi and Hussain [1], the formability improvement of a Cu/steel bimetal sheet during SPIF was better than that in the stamping process due to the limitation of the delamination in the former process. In their further work [2], the relation between the maximum forming angle and the process parameters of the tri-layer Cu/steel/Cu was studied experimentally. The results of the study revealed that a complex relation was observed between the operating parameters of the tri-layer sheet. Gheysarian and Honarpisheh [3] investigated the effect of the layer arrangement, tool path, and tool diameter on formability (i.e., fracture depth) and surface quality of Al/Cu bimetal sheets. The results showed the improvement in the formability corresponding to a large tool diameter, spiral tool path, and copper layer as a contacted sheet. Later, Honarpisheh et al. [4] focused on the improvement of the maximum forming angl...