Ar/ 39 Ar thermochronologic data from an extensional detachment zone in western Norway document punctuated late Paleozoic through Mesozoic tectonothermal activity. Diffusion and thermal modeling of alkali feldspars sampled in a profile through the detachment replicate laboratory argon release patterns when feldspars comprise three or four diffusion domains with differing activation energies that represent high-, intermediate-, and low-closure temperatures. These domains correspond to distinct changes in late Paleozoic cooling rates: (1) slow cooling at 0.4Њ-2.2ЊC/m.yr. from ca. 380-360 Ma; (2) rapid cooling at ≥15ЊC/m.yr. in Late Devonian-Early Carboniferous time (360-340 Ma); (3) slow cooling at 0.4Њ-1.7ЊC/m.yr. after ca. 340 Ma, with partial argon loss in Permian and Late Jurassic-Early Cretaceous times. The Early Carboniferous rapid cooling event recorded by the feldspars links the western Norway margin to contemporaneous unconformities, regional extension, basin inversion, and igneous activity previously identified around the proto-North Atlantic perimeter. We attribute this Early Carboniferous rapid cooling event in western Norway to an episode of unroofing. Unroofing was a consequence of increased topography and erosion; movement of the rocks toward the surface (higher topography) may have been triggered by thermal underplating combined with regional, transcurrent tectonics. The results support the judicious application of multidiffusion domain analysis of Ar-Ar alkali feldspar data from areas with well-constrained tectonostratigraphy and other, independent means of age control.