The piezo-phototronic effect uses the piezoelectric potential/piezoelectric
charge generated by the piezoelectric semiconductor material to regulate
the energy band structure and photogenerated carrier behavior at the
interface/junction, thereby modulating the device’s performance.
The positive/negative piezoelectric charges generated at the interface
of piezoelectric semiconductors can reduce the electron/hole barriers
and thus enhance the transport of photogenerated carriers. However,
electron/hole potential wells are formed when the electron/hole potential
barrier caused by positive/negative piezoelectric charges is lowered
too much, hindering the transport of photogenerated carriers. It is
difficult to balance the relationship between potential barriers and
potential wells while introducing the piezo-phototronic effect. In
this work, a physical mechanism by separating the photosensitive layer
and the piezoelectric modulation layer is proposed to deal with the
above-mentioned issue in flexible tunneling devices. The piezoelectric
modulation layer is solely used to adjust the electron/hole barriers,
while the photosensitive layer is used to absorb photons and generate
photogenerated carriers. This avoids the limitation on the transport
of photogenerated carriers caused by potential wells in the piezoelectric
semiconductor, thereby significantly increasing the adjustable range
of the barriers. Experimental results show that the photoresponsivity
of the flexible p-Si/Al2O3/n-ZnO tunneling device is optimized from 5.5 A/W to 35.8 A/W by the
piezo-phototronic effect after separating the piezoelectric charges
and photogenerated carriers. In addition, finite element analysis
is used to simulate the influence of piezoelectric charges on the
energy bands to corroborate the accuracy of the theoretical mechanism
and experimental results. This work not only presents an optoelectronic
device with excellent performance but also offers novel guidance for
improving the performance of optoelectronic devices using the piezo-phototronic
effect.