Abstract.The potassium-argon age of the Sikhote AUn iron meteorite --9 has been determined. The value i s 1 . 7 + 0.2 x 10 years. Previous lead data suggest an age of 4.6 x 10' ye a r s . The date of solidification m q be the sum of these two ages.Lead isotopic r a t i o s showing an excess of the nuclides lead-206, -207, and -208 relative t o lead-204 have been measured i n several iron meteorites'').A s with such r a t i o s reported f o r stone meteorites, these excesses may represent radiogenic contributions f ram the natural decay of uranium-235, uranium-238, and !thorium-232, respectively. However, i n one of these meteorites, Sikhote Alin, an upper limit was s e t t o the abundance of uranium-235 such that the excess lead-207 10
Tk(2 could not be accounted f o r by uranium decay i n a period l e s s than 10 years . This represents t~o '~~e r s of magnitude too l i t t l e uranium t o agree with the calcu-
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9(3 lated lead-lead age of 4.6 x 10 yeaxs .A possible explanation for t h i s uraniun deficiency would be a recent melting and chemical fractionation of the material t h a t i s now the Sikhote AUn meteorite.A suitable method of testing t h i s hypothesis i s by means of potassium-argon dating, since any process capable of removing uranium frcm the meteoritic mass w o u l d also remove the argon. Such an experiment fa reported here, and leads t o a potassium-9 argon "age" of abuut 1 . 7 x 10 yews. This i s significantly less than such ages previausly measured f co. other iron meteorites"),and mqy indicate that a recent melting (or at l e a s t a severe heating) did occur. This i s a necessary but not a suff'icient condition f o r the removal of uranium froan lead.Three separate runs were nade at the Brookhaven Reactor, i n which samples 3-5 2 grams i n size were irradiated f o r three ho~&s a t a flux of 5 x 1 0~ n/m see. ,
DISCLAIMERPortions of this document may be illegible in electronic image products. Images are produced from the best available original document.was placed i n an alumina crucible i n a vacuum l i n e , then boiled by induction heating f o r twenty minutes i n the presence of argon c a r r i e r . The evolved gases were gassed over hot titanium, which was then cooled t o remove hydrogen. The gases were then pumped i n t o a proportional counter with a background of about 10 counts per minute. The chemical y i e l d was 100% i n a l l cases. I n i t i a l counting r a t e s i n t h e three samples varied from 4000 t o 300 counts per minute. The a c t i v i t y followed the argon-41 h a l f -l i f e down t o about 15 cpm, then decayed with the argon-37 h a l f -l i f e be made from the argon-37 a c t i v i t y , which r e s u l t s from the ArJ6(n, r)Ar37 reaction.~r g o n -3 6 i s produced i n meteorites through d i r e c t nuclear production and through the decay of cosmic ray produced chlorine-36. The cross section r a t i o , from i r o n t a r g e t s , of (Ar36 + C 1 3 6 ) /~4 0 i s about 5 ( 5 ) . The correction f o r cosmogenic argon-40 i n this meteorite amounts t o about ...