We quantify the effective radiative forcing (ERF) of anthropogenic aerosols modelled by the aerosol-climate model CAM5.3-MARC-ARG. CAM5.3-MARC-ARG is a new configuration of the Community Atmosphere Model version 5.3 (CAM5.3) in which the default aerosol module has been replaced by the two-Moment, Multi-Modal, Mixing-stateresolving Aerosol model for Research of Climate (MARC). CAM5.3-MARC-ARG uses the default ARG aerosol activationscheme, consistent with the default configuration of CAM5.3. We compute differences between simulations using year-1850 aerosol emissions and simulations using year-2000 aerosol emissions in order to assess the radiative effects of anthropogenic aerosols. We compare the aerosol column burdens, cloud properties, and radiative effects produced by CAM5.3-MARC-ARG with those produced by the default configuration of CAM5.3, which uses the modal aerosol module with three lognormal modes (MAM3). Compared with MAM3, we find that MARC produces stronger cooling via the direct radiative effect, stronger cooling via the surface albedo radiative effect, and stronger warming via the cloud longwave radiative effect.The global mean cloud shortwave radiative effect is similar between MARC and MAM3, although the regional distributions differ. Overall, MARC produces a global mean net ERF of W m -2 , which is stronger than the global mean net ERF of W m -2 produced by MAM3. The regional distribution of ERF also differs between MARC and MAM3, largely due to differences in the regional distribution of the cloud shortwave radiative effect. We conclude that the specific representation of aerosols in global climate models, including aerosol mixing state, has important implications for climate modelling.
IntroductionAerosol particles influence the earth's climate system by perturbing its radiation budget. There are three primary mechanisms by which aerosols interact with radiation. First, aerosols interact directly with radiation by scattering and absorbing solar and thermal infrared radiation (Haywood and Boucher, 2000). Second, aerosols interact indirectly with radiation by perturbing clouds, by acting as the cloud condensation nuclei on which cloud droplets form and the ice nuclei that facilitate freezing of cloud droplets (Fan et al., 2016;Rosenfeld et al., 2014): for example, an aerosol-induced increase in cloud cover would lead to increased scattering of "shortwave" solar radiation and increased absorption of "longwave" thermal infrared radiation. Third, aerosols can influence the albedo of the earth's surface (Ghan, 2013): for example, deposition of absorbing aerosol on snow reduces the albedo of the snow, causing more solar radiation to be absorbed at the earth's surface.The "effective radiative forcing" (ERF) of anthropogenic aerosols, defined as the top-of-atmosphere radiative effect caused by anthropogenic emissions of aerosols and aerosol precursors, is often used to quantify the radiative effects of aerosols (Boucher et al., 2013). The anthropogenic aerosol ERF is approximately equivalent to "the rad...