On ultrafast x-ray scattering methods for magnetism

Plumley, R.; Chitturi, S. R.; Peng, C.; Assefa, T. A.; Burdet, N.; Shen, L.; Chen, Z.; Reid, A. H.; Dakovski, G. L.; Seaberg, M. H.; O’Dowd, F.; Montoya, S. A.; Chen, H.; Okullo, A.; Mardanya, S.; Kevan, S. D.; Fischer, P.; Fullerton, E. E.; Sinha, S. K.; Colocho, W.; Lutman, A.; Decker, F.-J.; Roy, S.; Fujioka, J.; Tokura, Y.; Minitti, M. P.; Johnson, J. A.; Hoffmann, M.; Amoo, M. E.; Feiguin, A.; Yoon, C.; Thayer, J.; Nashed, Y.; Jia, C.; Bansil, A.; Chowdhury, S.; Lindenberg, A. M.; Dunne, M.; Blackburn, E.; Turner, J. J.

doi:10.1080/23746149.2024.2423935

Advances in Physics: X

2024

DOI: 10.1080/23746149.2024.2423935

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On ultrafast x-ray scattering methods for magnetism

R. Plumley,

S. R. Chitturi,

C. Peng

et al.

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2024

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3D Heisenberg universality in the van der Waals antiferromagnet NiPS3

Plumley,

Mardanya,

Peng

et al. 2024

npj Quantum Mater.

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Van der Waals (vdW) magnetic materials are comprised of layers of atomically thin sheets, making them ideal platforms for studying magnetism at the two-dimensional (2D) limit. These materials are at the center of a host of novel types of experiments, however, there are notably few pathways to directly probe their magnetic structure. We confirm the magnetic order within a single crystal of NiPS3 and show it can be accessed with resonant elastic X-ray diffraction along the edge of the vdW planes in a carefully grown crystal by detecting structurally forbidden resonant magnetic X-ray scattering. We find the magnetic order parameter has a critical exponent of β ~ 0.36, indicating that the magnetism of these vdW crystals is more adequately characterized by the three-dimensional (3D) Heisenberg universality class. We verify these findings with first-principles density functional theory, Monte-Carlo simulations, and density matrix renormalization group calculations.

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3D Heisenberg universality in the van der Waals antiferromagnet NiPS3

Plumley,

Mardanya,

Peng

et al. 2024

npj Quantum Mater.

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show abstract

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On ultrafast x-ray scattering methods for magnetism

Cited by 1 publication

References 167 publications

3D Heisenberg universality in the van der Waals antiferromagnet NiPS3

3D Heisenberg universality in the van der Waals antiferromagnet NiPS3

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